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publication name Mechanically robust, electrically and thermally conductive graphene-based epoxy adhesives
Authors Qingshi Meng, Sensen Han, Sherif Araby, Yu Zhao, Zhiwen Liu, Shaowei Lu
year 2019
keywords Graphene; epoxy adhesives; electrical conductivity; lap shear strength
journal Journal of Adhesion Science and Technology
volume 33
issue 12
pages 1337-1356
publisher Taylor & Francis
Local/International International
Paper Link https://www.tandfonline.com/doi/full/10.1080/01694243.2019.1595890
Full paper download
Supplementary materials Not Available
Abstract

This study develops a facile approach to fabricate adhesives consists of epoxy and cost-effective graphene platelets (GnPs). Morphology, mechanical properties, electrical and thermal conductivity, and adhesive toughness of epoxy/GnP nanocomposite were investigated. Significant improvements in mechanical properties of epoxy/GnP nanocomposites were achieved at low GnP loading of merely 0.5 vol%; for example, Young’s modulus, fracture toughness (K1C) and energy release rate (G1C) increased by 71%, 133% and 190%, respectively compared to neat epoxy. Percolation threshold of electrical conductivity is recorded at 0.58 vol% and thermal conductivity of 2.13 W m−1 K−1 at 6 vol% showing 4 folds enhancements. The lap shear strength of epoxy/GnP nanocomposite adhesive improved from 10.7 MPa for neat epoxy to 13.57 MPa at 0.375 vol% GnPs. The concluded results are superior to other composites or adhesives at similar fractions of fillers such as single-walled carbon nanotubes, multi-walled carbon nanotubes or graphene oxide. The study promises that GnPs are ideal candidate to achieve multifunctional epoxy adhesives.

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